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Angular redistribution of near-infrared emission from quantum dots in 3D photonic crystals

机译:3D光子晶体中量子点的近红外发射的角度重新分布

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摘要

We study the angle-resolved spontaneous emission of near-infrared light sources in three-dimensional photonic crystals over a wavelength range 1200–1550 nm. To this end, PbSe quantum dots are used as light sources inside titania inverse opal photonic crystals. Strong deviations from the Lambertian emission profile are observed. An attenuation of 60% is observed in the angle-dependent radiant flux emitted due to photonic stop bands. At angles that correspond to the edges of the stop band, the emitted flux is increased by up to 34%. This increase is explained by the redistribution of Bragg-diffracted light over the available escape angles. The results are quantitatively explained by an expanded escape-function model. This model is based on diffusion theory and adapted to photonic crystals using band structure calculations. We identify the need to separately consider the transport mean free path of both the emitted light and the light used for excitation. Here, the model is applied to describe emission in the regime where samples are optically thick for the excitation light, yet relatively thin for the photoluminesence light
机译:我们研究了在波长为1200-1550 nm的三维光子晶体中近红外光源的角度分辨自发发射。为此,将PbSe量子点用作二氧化钛反蛋白石光子晶体内部的光源。观察到与朗伯排放曲线的强烈偏差。由于光子阻带,在与角度相关的辐射通量中观察到60%的衰减。在对应于阻带边缘的角度处,发射通量最多增加34%。这种增加可以通过布拉格衍射光在可用逸出角上的重新分布来解释。结果由扩展的逃逸函数模型定量解释。该模型基于扩散理论,并通过能带结构计算适用于光子晶体。我们确定有必要分别考虑发射光和用于激发的光的传输平均自由程。在这里,该模型用于描述在以下情况下的发射:对于激发光,样品的光学厚度是光学上的,而对于光致发光的光,样品则相对较薄

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